By Flemming Ove Olsen
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B. Corrosion, 1984, 40(12), 663-668. 55. Lesinski, C. A. S. Patent 3,308,065, 1967. 56. Harriman, L. W. etal. US. 81 1, 1969. 57. Alfano, S . S. Patent 3,072,502, 1963. 58. Bell, W. E. S. Patent 3,248,269, 1966. 59. Pitzer, E. C. US. Patent 3,297,580, 1967. 60. Johnson, A. B. et a/. Paper 38, presented at the 33rd Corrosion Forum, NACE International: Houston, TX, 1978. 61. Pettit, P. ; McTgue, P. F. Paper 208, presented at the 33rd Corrosion Forum, NACE International: Houston, TX, 1978. 62. Martell, A.
Mundis, J. A. Presented at the American Power Conference: Chicago, IL, 1982. 46. Bradbury, 0. et al. Presented at the Conference on Decontamination of Nuclear Facilities, LaGrange Park, IL, 1982; pp. 3-21. 47. ; Azuma, K. Trans. AIM€, 1968, 24(2), 1025. 48. ; Ferrier, A. Rep. RE438, Institut des Recherches de la Siderurgie Franchise: St. Germainen-Laye, France, 1977. 49. Fields, W. M. Presented at the 2nd International Congress on Metallic Corrosion: Houston, TX, 1963. 50. McPherson, W. ; Martin, J.
33) rate determining CHAPTER 3: Mechanisms of Iron Oxide and Copper Dissolution 47 The major oxidizing agent for the EDTA system is Fe(lll)EDTA,while the external oxidizer (oxygen, nitrite) oxidizes the copper in the iron citrate system. The external oxidizer does oxidize the ferrous citrate to ferric citrate, but this species does not dissolve much of the copper; it actually acts as a sink for the external oxidizer. The only benefit of using the iron citrate solution is that an additional oxidizing fill of the unit is avoided.
